Professional Legacy

An Article by Peter Miodownik

Appreciation of Larry Kaufman Lifetime Achievement V2  10/08/11

My personal contact with Larry started about forty years ago, around the time that the idea  of Calphad community first came into being. I had come into contact with his work some ten years earlier, but papers are dry and desiccated things compared to personal contact! At that time he was still largely an unrecognised pathfinder, ploughing a relatively lonely furrow, but continually hopeful for the future.  It was, and is, rare to find someone with such a single-minded determination and a great privilege to watch his early work come to fruition in such a spectacular way.

In these days of incredibly powerful personal computers it is sobering to realise that the seeds of the Calphad Procedure lay in an aged and creaking IBM machine fed with punched cards and whose limited powers severely restricted the functions that could be programmed.  It was however sufficient to allow Larry to carry through the brilliant idea  that a list of standardised phase stabilities for each crystallographic arrangement could be made the keystone of a new thermodynamic approach, at a time when it was not at all commonplace to consider that all elements were capable of allotropy under the right circumstances.  It was really exciting to see living proof that ideas are more important than the available hardware for the development of new paradigms, although it is clear that smarter electronics.have enabled all of us to push the boundaries of the Calphad Technique ever forward.

Throughout the time I have known him, Larry has always been an impressive net-worker with his colleagues all over the world.  An indefatigable letter-writer, mostly writing by hand in a characteristic style, filling every available space annotating text with  comments on every available margin.  This tendency  spilled over into a rather idiosyncratic method of  using a rapid succession of overheads. These were so densely packed with information that it was sometimes very difficult  to absorb, or even see, what was being displayed before it was replaced by another equally dense set of data.

I was fortunate to have been given access his private correspondence which shows how difficult it was to shift the phase diagram community away from its pre-occupation with electron-atom ratios and band theory as construed at the time.  He corresponded tirelessly with proponents of the electron theory current at the time, such as William Hume-Rothery and Leo Brewer, who did not believe in the values of the phase stabilities nor that a combination of such values could be successfully married with simple solution models.

This battle continued for decades  It is truly remarkable that Larry was never discouraged by this opposition; he just patiently chipped away at their objections, firm in the knowledge that they would come round to see that his point of view was ultimately based on experimental evidence and that all theoretical approaches needed to examine their assumptions. Larry was in fact always very keen that agreement should be reached between various approaches and an extended correspondence with David Pettifor  was followed by the suggestion that I should visit  him at the Cavendish Laboratory where he was working at the time. That encounter gradually led to an increasing number of physicists attending Calphad Meetings and an eventual resolution of the differences that had divided the two communities for such a long time

The current international nature of CALPHAD is taken for granted, but in the early days political battles had to be fought to obtain funds for even just bi-lateral collaboration. It is not usually realised that, quite apart from his role as the initiator of the Calphad Approach, Larry also spent a great deal of time behind the scenes to acquire and manage the necessary funds required to kick-start the Calphad Meetings. All those who have organised such meetings will know that it is virtually impossible without the knowledge that there is financial backing to make advance bookings and subsidise key speakers.

Larry was, of course, also the major force behind the concept of a journal which would demonstrate the power of the Calphad method. It was no easy task to persuade Pergammon that there was going to be a sufficient market based  on a new methodology, with which the scientific community was not entirely in agreement at that time. Moreover as editor in chief for a long time, he had to make sure that the proofs of each copy was delivered on time and monitor the standard of the papers.

None of this could have happened without Larry’s great capacity for multi-tasking. He really was capable of handling many problems simultaneously. I particularly remember Harvey Nesor shouting from the room next door that a set of parameters for some new system were not working.  Larry suggested some new values while at the same time answering the telephone and conducting a conversation with me across the desk. He always had a fantastic feeling for the right orders of magnitude of various thermodynamic properties regardless of whether it was a well known system or something he was tackling for the first time.

During my spell at ManLabs, Larry also demonstrated  another form of multitasking and showed that  time could be persuaded to multiply itself by easting and working simultaneously.
 
Larry was always convinced that there was no system that could not be handled, no metastable condition that could not be incorporated, and no boundaries between subjects such as chemistry, geology physics and ceramics. Practioners in all these fields were invited to Calphad Meetings at one time or another. His thorough grasp of the unity underlying thermodynamic parameters meant that he was a past-master at coupling apparently unrelated information and extracting missing parameters to his data base. The relatively neglected pressure variable is a case in point. Applications in the field of martensitic  transformation  and even radiation damage became fruitful areas of research and led to my own research group to successfully apply the calphad approach  to that most metastable condition of them all, namely amorphous alloys.

LK was quite happy to take on board developments in methodology which required a substantial switch from the model with which he started. He really enjoyed the  developments made under the guidance of his old friend Mats Hillert at RTI in Stockholm as this allowed a major expansion in the number of elements that could be handled simultaneously and was also far more user-friendly.

Retirement is of course a word that is not in Larry’s vocabulary. He must be one of the few people who voluntarily spend part of their “retirement” By entering an academic institution [MIT] rather than retiring  FROM it….


http://www.calphad.org/


It is with utmost sadness that we announce the passing of Dr. Larry Kaufman on December 2 in Israel. He was the founder of CALPHAD, the father of Materials Genome, our mentor, colleague, and dear friend.

Flowers/cards/letters can be sent to

Valerie Farber c/o Sandra Kaufman

Har Nevo St.

         Hashmonaim Israel 73127

 

The CALPHAD Board is working on establishing a scholarship fund under his name and publishing a special CALPHAD issue dedicated to him. More information to come.



It is with profound sadness and grief that I and the computational thermodynamics fraternity of India receive the news of the passing away of Dr. Larry Kaufman. For several generations to come, Dr Larry Kaufman will be remembered for his outstanding contributions towards the evolution of the CALPHAD method. The invention of the organized and structured CALPHAD method was a stroke of genius and only today are we able to realize its full potential with the advent of Integrated Computational Materials Engineering. He could think far ahead of his times.

I and all of my colleagues at CSIR-NML pay our deepest condolences to him and pray for his departed soul to rest in peace.

Regards

S.Srikanth

Director
National Metallurgical Laboratory
Jamshedpur - 831 007, India
Tel: +91-657-2345202/2345028   Fax: +91-4657-2345213



Sorry to hear about Larry Kaufman. He was an amazing visionary. His passing will create a void at future CALPHAD meetings.
Best regards,
John Morral




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